Coherent Harmonic Generation on UVSOR-II storage ring

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CEA / Service des Photons Atomes et Molécules Coherent Harmonic Generation on UVSOR-II storage ring M. Labat, C. Bruni, G. Lambert, M. Hosaka, A. Mochihashi, M. Shimada, Y. Takashima, M. Katoh, T. Hara, K. Fukui, M.E. Couprie. Acknowledgments: S. Bielawski, C. Szwaj, J. Yamazaki.

CHG FEL configuration Optical klystron Seeding Laser FEL pulse or External laser λ λ λ/n Coherent Harmonic Generation λ/(n.h) (1) Energy modulation (3) Coherent radiation (2) Density modulation

CHG FELs background CHG first proposed in 1982 R. Coïsson and F. De Martini, Phys. Of Quant. Elec. 9 (1982). CHG with external seed: First demonstration on ACO storage ring: R. Prazeres et al., NIM A272 (1988). Nd:Yag laser (1064.1 nm) seeded in OK Generation of H3 (354.7 nm) of fund. Generation of H3 (177 nm) and H5 (106.4 nm) of doubled laser Similar results on: Super ACO storage ring: R. Prazeres et al., NIM A304 (1991). MAX-lab storage ring: S. Werin et al., NIM A290 (1990). Present experiments (using Ti:Sa laser at 800 nm): @ UVSOR-II M. Labat et al., Euro. Phys Jour. D 44 (2007) 187. @ ELETTRA F. Curbis et al., FEL 07. CHG with internal seed (FEL pulse stored in a cavity): @ DUKE: V. Litvinenko et al., NIM A507 (2003). at 665.4 nm H3 (221.8 nm) at 236 nm H2 to H7 (118 to 37 nm) @ ELETTRA: at 660 nm gives H3 (220 nm) G. De Ninno, Proc. FEL 04 (2004) 237.

CHG and HGHG FELs CHG FELs on SR: Limited undulator length + Limited beam quality Limited power HGHG FELs: L.H. Yu et al., Science 489 (2000). Long undulators saturation power ~ GW Short wavelengths Good coherence Future FEL sources (Arc-En-Ciel, BESSY-FEL, Fermi, 4GLS, MAX-Lab, ) Common issues: Seeding techniques: synchronisation, alignement Seeding energy level to overcome shot noise Coherence improvement from seeding Nonlinear harmonic generation Investigations on CHG FELs can be useful for future FELs sources GW @ ~ 1nm

CHG experiments on UVSOR-II SR Streak Camera SR @ 5.6 MHz UVSOR-II e- beam 600 MeV, 90 ps-rms, f rev =5.6 MHz / T rev =178 ns Bending magnet RF cavity 100 kv, 90.1 MHz Optical Klystron 2 Undulators + 1 Dispersive Section 9 periods of 11 cm UVSOR-II FEL Seeding Laser Ti:Sa, 800 nm, 1.5 W, 1.2 ps-fwhm, 1 khz CHG @ 1 khz H2: 400 nm, H3: 266 nm, H4: 200 nm Commercial system: Mode-locked Ti:Sa oscillator (Coherent, Mira 900-F), and Regenerative amplifier (Coherent, Legend HE)

1 st result: Coherent Generation of H3 (266 nm) CHG CHG Quadratic fit I=2.5 ma H3 with CHG = H3 SE x 5 CHG α I peak ²: signature of coherence M. Labat et al., Euro. Phys Jour. D 44 (2007) 187.

Beam dynamics studies (1) Simulation of e- distribution: Beam heating Saturation Double oscillating structure: Laser repetition rate Synchrotron frequency Equilibrium state depends on laser parameters possible adjustment of heating optimisation of average/peak Exp. measurement: Bunch lengthening ~ 10 % f=100 Hz f=1 khz f=10 khz Qualitative agreement with simulations M. Labat et al., submitted to Eur. Phys. Lett. In July 2007.

Beam dynamics studies (2) Simulation of beam profile evolution: At each injection (i): Hole (< 10 turns life time) Progressive diffusion Progressive lengthening Laser off At saturation: i-5 1 st injection At saturation: i+1 Saturation comes from LOCAL HEATING Rep rate= 1 khz, P=5 W, pulse duration= 6 ps-fwhm.

CHG Transverse Coherence Young slits experiment: 2D interference pattern Visibility of the fringes Mutual coherence degree Transverse coherence 2D detector: Fast intensified CCD camera for CHG (harmonic pulse gating) Optical Klystron Young s Slits Lens UV filter BP filter ND filter Detector

CHG transverse coherence SE SE: V=0.33 CHG With seeding: Visibility: 0.33 0.7 CHG: V=0.7 Further FEL analysis undergoing in collaboration with G. Dattoli See Poster: TUPPH007

Even Harmonic Generation with planar undulators Oscillator FELs: Select efficient coupling coef. between transverse cavity modes and harmonics M.J. Schmitt et al., PRA 34 (1986) 4843 Wave guides H. Bluem et al., PRL67 (1991) 824 CHG FELs: No cavity no possible mode selection SE even harmonics: off-axis CHG even harmonics expected: strong off axis radiation

Even Harmonic Generation with planar undulators Exp. setup: Optical Klystron PM 1 R928 BP filters @ 405 nm T 405 nm = 50 % T 800 nm = 0.01% PM 2 R729 (Solar blind) BP filter @ 200 nm T 200 nm = 12 % T 800 nm = 0.01 % 1 st results: CHG H2: SE x 3.6 H4: SE x 2 Low pass filter Laser Laser

Even Harmonic Generation with planar undulators Angular distribution of H2: Clear off-axis distribution Transverse scan with a 3 mm pinhole Pinhole aperture (mm)

Even Harmonic Generation with planar undulators Comparison to SE calculated with SRW & SPECTRA. CHG appears: More divergent To be confirmed with MEDUSA simulations (H. Freund, Private Communications) SRW SPECTRA

CHG with helical undulators Helical undulators enable: Circular polarisation various users experiments Debated issue: Azymuthal resonance HG on-axis Usual resonance HG off-axis H.P. Freund et al., PRL 94 (2005). G. Geloni et al., Opt. Comm. 271 (2007).

CHG with helical undulators Experimental setup @ UVSOR: OK helical configuration e- beam E=500 MeV for resonance matching @ 800 nm Laser variable polarisation using a λ/4

CHG with helical undulators Results: Coherent Harmonic Generation on H2: H2 intensity = SE x 3 Still CHG on H3 I=2.8 ma

CHG with helical undulators Angular distribution of H2: Off-axis Laser polarisation dependency of H2: (L) max CHG (C) min CHG Expected/Unpexted Further checking on: CHG Alignment Over bunching Next: HG efficiency vs n H (L) (L) (L) SE (C) (C) (C) (C) To be compared with both approaches expectation I=1 ma

Conclusion Experimental work on CHG FEL @ UVSOR-II: Beam dynamics under laser heating Seeding effect on transverse coherence Harmonic Generation possibilities: * Even HG * HG with helical undulators Step forward in CHG FEL understanding Encouraging/Useful results for HGHG FELs

CHG energy per pulse Calculation of SE level with SPECTRA: 1.8 pj @ 2.4 ma on detector 7.2 pj before filter Amplification of SE by factor 5 Estimation of CHG energy: SE x 5 x 2.4 CHG ~ 87.5 pj CHG ~ 0.1 µj

Longitudinal coherence Longitudinal coherence: * Pulse length: < 3 ps-rms (SC resolution) * Spectral width: < 2.5 nm (spectrometer resolution)

CHG intensity optimisation Systematic measurements versus: Undulator gap Laser parameters (power, pulse duration, diameter) Optimisation of H3 CHG P=1.6 W P=0.8 W SR

Harmonic Generation Future investigations : Compare planar/helical configurations in terms of : HG efficiency vs n H

BP filter @ 400 nm: * Opto sigma corporation: VPF-25C-40-40-4000 Centered @ 405 nm Δλ fwhm =40 nm T 405 nm =50 % T 800 nm =0.01% * Corion: P10405A-H972 Centered @ 405 nm Δλ fwhm =10 nm T 405 nm =50 %?? T 800 nm =0.01% Low pass filter: Sigma Kouki UTVAF-50S-34U T λ<340 nm < 0.01 % BP filter @ 200 nm: MA200nm T 200nm = 12 % Δλfwhm=10 nm T 800nm = 0.01%

Dear Marie-san, Actually the filter is very old one and I do not know from which company it is bought. Yesterday I checked removing from the filter holder and found it is just labeled "MA200nm". The filter size is 30mm and we have a lot of similar ones. I am not very sure but the typical values of specification of that kind of filters are Peak transmission 12% Band width FWHM = 10nm I think in case of the filter @200 nm these values is not far. Best Regar

Dear Marie-san, The reference of the filter is Sigma Kouki UTVAF-50S-34U You can find information of the filter here. http://www.sigmakoki.com/english/b/filters/coloredglassfilters/utvaf/utvaf.html#0. The 200 nm filter is very old one and I am not sure that I can find the reference. Best regards, Masahito Hosaka